Sending Mail Stopped Working

“Cannot connect to server” means just that. Your device is not able to connect to the remote server.

The server name is correct and works for me. That leaves a network error as likely source of the problem. If I had to guess, I’d say it’s IPv6-related. The fallback to IPv4 isn’t working properly in the current stable version of K-9 Mail (6.202). Try using the latest beta version. See How do I become a beta tester?